Xu Yunting, Zhang Kai, Dai Xiaoye, et al. Mechanism and Experimental Studies of HFC-134a Oxidative Decomposition Mechanism[J]. Journal of refrigeration, 2023, 44(3).
DOI:
Xu Yunting, Zhang Kai, Dai Xiaoye, et al. Mechanism and Experimental Studies of HFC-134a Oxidative Decomposition Mechanism[J]. Journal of refrigeration, 2023, 44(3). DOI: 10.3969/j.issn.0253-4339.2023.03.029.
Mechanism and Experimental Studies of HFC-134a Oxidative Decomposition Mechanism
There is significant emphasis on the destruction of HFC refrigerants in China
culminating in an urgent need to explore efficient and mild HFC refrigerant degradation methods. In this study
a typical HFC refrigerant
HFC-134a
was chosen as the object of combined experimental studies and quantum chemical calculations
and the degradation rate was considered the main criterion for exploring the high-level pathway of refrigerant degradation. In terms of quantum chemistry
the reaction paths of HFC-134a under pyrolysis and oxidative decomposition conditions were explored. Under both paths
detectable stable products such as CHF=CF2 and HF were easily produced. During pyrolysis
the first step in the chemical bond cleavage is the rate-determining step. Compared to the pyrolysis path
the oxidative decomposition path has a lower reaction energy barrier
which is conducive to the rapid occurrence of the reaction. Experimental results showed that the degradation rate of HFC-134a increased from 11% to 66% with the increase in temperature in the range of 240–360 ℃. By fitting the kinetic constant of the reaction
the pre-exponential factor (A) of HFC-134a was determined as 7471.04 s-1
and the activation energy (Ea) was 54.16 kJ/mol
which were consistent with the simulated chemical reaction energy barrier.